Is it possible to use the Organelle as an audio interface for my iMac and use it as a recorder for recording live jams?
no its not an audio interface.
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You can record you jams with it though! Look up the ‘recorder’ patch by critter and guitari.
I tried. The organelle froze 
It might be missing the required Sounds folder in the patch folder. Try downloading a new version:
http://thepeacetreaty.org/organelle/patches/Recorder.zip
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